Imperial College London

Professor SirJohnPendry

Faculty of Natural SciencesDepartment of Physics

Chair in Theoretical Solid State Physics
 
 
 
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Contact

 

+44 (0)20 7594 7606j.pendry CV

 
 
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Assistant

 

Mrs Carolyn Dale +44 (0)20 7594 7579

 
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Location

 

808Blackett LaboratorySouth Kensington Campus

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Summary

 

Publications

Citation

BibTex format

@article{Demetriadou:2017:10.1021/acsphotonics.7b00437,
author = {Demetriadou, A and Hamm, J and Luo, Y and Pendry, J and Baumberg, J and Hess, O},
doi = {10.1021/acsphotonics.7b00437},
journal = {ACS Photonics},
pages = {2410--2418},
title = {Spatio-temporal dynamics and control of strong coupling in plasmonic nano-cavities},
url = {http://dx.doi.org/10.1021/acsphotonics.7b00437},
volume = {4},
year = {2017}
}

RIS format (EndNote, RefMan)

TY  - JOUR
AB - In the light-matter strong coupling regime, the excited state of quantum emitters is inextricably linked to a photonic mode, leading to hybrid states that are part-light and part-matter. Recently, there has been huge effort to realize strong coupling with nanoplasmonics, since it provides a versatile environment to study and control molecules in ambient conditions. Amongst the most promising designs are plasmonic nano-cavities that confine light to unprecedentedly small volumes. Such nano-cavities though support multiple types of modes, with different field profiles and radiative decay rates (bright and dark modes). Here, we show theoretically that the different nature of these modes leads to mode beating within the nano-cavity and the Rabi-oscillations, which alters the spatio-temporal dynamics of the hybrid system. By specifically designing the illumination set-up, we decompose and control the dark and bright plasmon mode excitation and therefore their coupling with quantum emitters. Hence, this work opens new routes for dynamically dressing emitters, to tailor their hybrid states with external radiation.
AU - Demetriadou,A
AU - Hamm,J
AU - Luo,Y
AU - Pendry,J
AU - Baumberg,J
AU - Hess,O
DO - 10.1021/acsphotonics.7b00437
EP - 2418
PY - 2017///
SN - 2330-4022
SP - 2410
TI - Spatio-temporal dynamics and control of strong coupling in plasmonic nano-cavities
T2 - ACS Photonics
UR - http://dx.doi.org/10.1021/acsphotonics.7b00437
UR - http://hdl.handle.net/10044/1/50593
VL - 4
ER -