Citation

BibTex format

@article{Xu:2022:10.1016/j.xcrp.2022.100890,
author = {Xu, W and Du, T and Sachs, M and Macdonald, TJ and Min, G and Mohan, L and Stewart, K and Lin, C-T and Wu, J and Pacalaj, R and Haque, SA and McLachlan, MA and Durrant, JR},
doi = {10.1016/j.xcrp.2022.100890},
journal = {Cell Reports Physical Science},
pages = {1--17},
title = {Asymmetric charge carrier transfer and transport in planar lead halide perovskite solar cells},
url = {http://dx.doi.org/10.1016/j.xcrp.2022.100890},
volume = {3},
year = {2022}
}

RIS format (EndNote, RefMan)

TY  - JOUR
AB - Understanding charge carrier extraction from the perovskite photoactive layer is critical to optimizing the design of perovskite solar cells. Herein, we demonstrate a simple time-resolved photoluminescence method to characterize the kinetics of charge transport across the bulk perovskite and charge transfer from the perovskite layer to the interlayers, elucidating the dependence of these dynamics on film thickness, grain boundaries (GBs), and interlayers. Using asymmetric laser excitation, we selectively probe charge transport by generating charges both close to and far from the heterojunction interface and correlate these results with device performance. We observe that both film thickness and GBs affect the asymmetry between electron and hole charge transport across the bulk perovskite and charge transfer from the bulk perovskite to the respective interlayers.
AU - Xu,W
AU - Du,T
AU - Sachs,M
AU - Macdonald,TJ
AU - Min,G
AU - Mohan,L
AU - Stewart,K
AU - Lin,C-T
AU - Wu,J
AU - Pacalaj,R
AU - Haque,SA
AU - McLachlan,MA
AU - Durrant,JR
DO - 10.1016/j.xcrp.2022.100890
EP - 17
PY - 2022///
SN - 2666-3864
SP - 1
TI - Asymmetric charge carrier transfer and transport in planar lead halide perovskite solar cells
T2 - Cell Reports Physical Science
UR - http://dx.doi.org/10.1016/j.xcrp.2022.100890
UR - https://www.sciencedirect.com/science/article/pii/S2666386422001680?via%3Dihub
UR - http://hdl.handle.net/10044/1/96757
VL - 3
ER -