Imperial College London
Prof. David Chadwick

Prof. David Chadwick

Faculty of Engineering, Department of Chemical Engineering

Professor
 
 
 
//

Contact

 

+44 (0)20 7594 5579d.chadwick

 
 
//

Location

 

235Roderic Hill BuildingSouth Kensington Campus

//

Summary

 

Publications

Citation

BibTex format

@article{Peng:2017:10.1016/j.jcou.2017.12.004,
author = {Peng, J and Iruretagoyena, Ferrer D and Chadwick, D},
doi = {10.1016/j.jcou.2017.12.004},
journal = {Journal of Co2 Utilization},
pages = {73--80},
title = {Hydrotalcite/SBA15 composites for pre-combustion CO2 capture: CO2},
url = {http://dx.doi.org/10.1016/j.jcou.2017.12.004},
volume = {24},
year = {2017}
}
Download

RIS format (EndNote, RefMan)

TY  - JOUR
AB  - Hydrotalcite-like compounds (HT) show potential as CO2 adsorbent materials for pre-combustion CO2 capture applications, but require improvements in stability, adsorption capacity and kinetics. In this study, HT/SBA15 hybrids (with different Mg/Al ratios varying from 0.3 to 3) have been synthesised using a two-stage grafting method to coat a mesoporous SBA15 with hydrotalcite layers. The HT/SBA15 hybrids showed significant improvement in intrinsic CO2 uptake (per mass of HT), initial uptake rate, and multicycle stability compared to unsupported HT. Compared to previously reported nanostructured carbon supports (e.g. CNF, MWCNTs), the HT/SBA15 hybrids were found to be more thermally stable and exhibit comparable adsorption uptake and rates. In particular, the use of SBA15 as a support is shown to prevent the gradual loss in weight from thermal decomposition observed for HT/MWCNT or HT/GO composites over extended cycling.
AU  - Peng,J
AU  - Iruretagoyena,Ferrer D
AU  - Chadwick,D
DO  - 10.1016/j.jcou.2017.12.004
EP  - 80
PY  - 2017///
SN  - 2212-9820
SP  - 73
TI  - Hydrotalcite/SBA15 composites for pre-combustion CO2 capture: CO2
T2  - Journal of Co2 Utilization
UR  - http://dx.doi.org/10.1016/j.jcou.2017.12.004
UR  - http://hdl.handle.net/10044/1/56874
VL  - 24
ER  -
Download