Imperial College London
Alternate

Professor Jon Marangos

Faculty of Natural Sciences, Department of Physics

Lockyer Chair in Physics
 
 
 
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Contact

 

+44 (0)20 7594 7857j.marangos Website

 
 
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Assistant

 

Ms Judith Baylis +44 (0)20 7594 7713

 
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Location

 

208Blackett LaboratorySouth Kensington Campus

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Summary

 

Publications

Citation

BibTex format

@article{Li:2021:1361-6455/abcdf1,
author = {Li, S and Driver, T and Al, Haddad A and Champenois, EG and Agaker, M and Alexander, O and Barillot, T and Bostedt, C and Garratt, D and Kjellsson, L and Lutman, AA and Rubensson, J-E and Sathe, C and Marinelli, A and Marangos, JP and Cryan, JP},
doi = {1361-6455/abcdf1},
journal = {Journal of Physics B: Atomic, Molecular and Optical Physics},
pages = {1--9},
title = {Two-dimensional correlation analysis for x-ray photoelectron spectroscopy},
url = {http://dx.doi.org/10.1088/1361-6455/abcdf1},
volume = {54},
year = {2021}
}
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RIS format (EndNote, RefMan)

TY  - JOUR
AB  - X-ray photoelectron spectroscopy (XPS) measures the binding energy of core-level electrons, which are well-localised to specific atomic sites in a molecular system, providing valuable information on the local chemical environment. The technique relies on measuring the photoelectron spectrum upon x-ray photoionisation, and the resolution is often limited by the bandwidth of the ionising x-ray pulse. This is particularly problematic for time-resolved XPS, where the desired time resolution enforces a fundamental lower limit on the bandwidth of the x-ray source. In this work, we report a novel correlation analysis which exploits the correlation between the x-ray and photoelectron spectra to improve the resolution of XPS measurements. We show that with this correlation-based spectral-domain ghost imaging method we can achieve sub-bandwidth resolution in XPS measurements. This analysis method enables XPS for sources with large bandwidth or spectral jitter, previously considered unfeasible for XPS measurements.
AU  - Li,S
AU  - Driver,T
AU  - Al,Haddad A
AU  - Champenois,EG
AU  - Agaker,M
AU  - Alexander,O
AU  - Barillot,T
AU  - Bostedt,C
AU  - Garratt,D
AU  - Kjellsson,L
AU  - Lutman,AA
AU  - Rubensson,J-E
AU  - Sathe,C
AU  - Marinelli,A
AU  - Marangos,JP
AU  - Cryan,JP
DO  - 1361-6455/abcdf1
EP  - 9
PY  - 2021///
SN  - 0953-4075
SP  - 1
TI  - Two-dimensional correlation analysis for x-ray photoelectron spectroscopy
T2  - Journal of Physics B: Atomic, Molecular and Optical Physics
UR  - http://dx.doi.org/10.1088/1361-6455/abcdf1
UR  - http://gateway.webofknowledge.com/gateway/Gateway.cgi?GWVersion=2&SrcApp=PARTNER_APP&SrcAuth=LinksAMR&KeyUT=WOS:000684385400001&DestLinkType=FullRecord&DestApp=ALL_WOS&UsrCustomerID=1ba7043ffcc86c417c072aa74d649202
UR  - https://iopscience.iop.org/article/10.1088/1361-6455/abcdf1
UR  - http://hdl.handle.net/10044/1/91323
VL  - 54
ER  -
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