Publications
142 results found
Hu H, Jackson MD, Blundy J, 2022, Melting, Compaction and Reactive Flow: Controls on Melt Fraction and Composition Change in Crustal Mush Reservoirs, JOURNAL OF PETROLOGY, Vol: 63, ISSN: 0022-3530
Jackson WA, Hampson GJ, Jacquemyn C, et al., 2022, A screening assessment of the impact of sedimentological heterogeneity on CO2 migration and stratigraphic-baffling potential: Johansen and Cook formations, Northern Lights project, offshore Norway, International Journal of Greenhouse Gas Control, Vol: 120, Pages: 103762-103762, ISSN: 1750-5836
We use a method combining experimental design, sketch-based reservoir modelling, and single-phase flow diagnostics to rapidly screen the impact of sedimentological heterogeneities that constitute baffles and barriers to CO2 migration in the Johansen and Cook formations at the Northern Lights CO2 storage site. The types and spatial organisation of sedimentological heterogeneities in the wave-dominated deltaic sandstones of the Johansen-Cook storage unit are constrained using core data from the 31/5-7 (Eos) well, previous interpretations of seismic data and regional well-log correlations, and outcrop and subsurface analogues. Delta planform geometry, clinoform dip, and facies-association interfingering extent along clinoforms control: (1) the distribution and connectivity of high-permeability medial and proximal delta-front sandstones, (2) effective horizontal and vertical permeability characteristics of the storage unit, and (3) pore volumes injected at breakthrough time (which approximates the efficiency of stratigraphic baffling). In addition, the lateral continuity of carbonate-cemented concretionary layers along transgressive surfaces impacts effective vertical permeability, and bioturbation intensity impacts effective horizontal and vertical permeability. The combined effects of these and other heterogeneities are also influential. Our results suggest that the baffling effect on CO2 migration and retention of sedimentological heterogeneity is an important precursor for later capillary, dissolution and mineral trapping.
Alarouj M, Jackson MD, 2022, Experimental measurement of the exclusion-diffusion potential in sandstone and shaly sand samples at full and partial water saturation, GEOPHYSICS, Vol: 87, Pages: M235-M246, ISSN: 0016-8033
Bahlali ML, Salinas P, Jackson MD, 2022, Efficient Numerical Simulation of Density-Driven Flows: Application to the 2-and 3-D Elder Problem, WATER RESOURCES RESEARCH, Vol: 58, ISSN: 0043-1397
Alshakri J, Hampson GJ, Jacquemyn C, et al., 2022, A screening assessment of the impact of sedimentological heterogeneity on CO2 migration and stratigraphic-baffling potential: Sherwood and Bunter Sandstones, UK, Geological Society, London, Special Publications, Vol: 528, ISSN: 0305-8719
We use a combination of experimental design, sketch-based reservoir modelling, and flow diagnostics to rapidly screen the impact of sedimentological heterogeneities that constitute baffles and barriers on CO2 migration in depleted hydrocarbon reservoirs and saline aquifers of the Sherwood Sandstone Group and Bunter Sandstone Formation, UK. These storage units consist of fluvial sandstones with subordinate aeolian sandstones, floodplain and sabkha heteroliths, and lacustrine mudstones. The predominant control on effective horizontal permeability is the lateral continuity of aeolian-sandstone intervals. Effective vertical permeability is controlled by the lateral extent, thickness and abundance of lacustrine-mudstone layers and aeolian-sandstone layers, and the mean lateral extent and mean vertical spacing of carbonate-cemented basal channel lags in fluvial facies-association layers. The baffling effect on CO2 migration and retention is approximated by the pore volume injected at breakthrough time, which is controlled largely by three heterogeneities, in order of decreasing impact: (1) the lateral continuity of aeolian-sandstone intervals; (2) the lateral extent of lacustrine-mudstone layers, and (3) the thickness and abundance of fluvial-sandstone, aeolian-sandstone, floodplain-and-sabkha-heterolith and lacustrine-mudstone layers. Future effort should be focussed on characterising these three heterogeneities as a precursor for later capillary, dissolution and mineral trapping.
Hamzehloo A, Bahlali ML, Salinas P, et al., 2022, Modelling saline intrusion using dynamic mesh optimization with parallel processing, ADVANCES IN WATER RESOURCES, Vol: 164, ISSN: 0309-1708
Regnier G, Salinas P, Jacquemyn C, et al., 2022, Numerical simulation of aquifer thermal energy storage using surface-based geologic modelling and dynamic mesh optimisation, HYDROGEOLOGY JOURNAL, Vol: 30, Pages: 1179-1198, ISSN: 1431-2174
Alarouj M, Jackson MD, 2022, Numerical modeling of self-potential in heterogeneous reservoirs, GEOPHYSICS, Vol: 87, Pages: E103-E120, ISSN: 0016-8033
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- Citations: 1
Collini H, Jackson MD, 2022, Relationship between zeta potential and wettability in porous media: insights from a simple bundle of capillary tubes model, Journal of Colloid and Interface Science, Vol: 608, Pages: 605-621, ISSN: 0021-9797
Hypothesis & MotivationExperimental data suggest a relationship between the macroscopic zeta potential measured on intact rock samples and the sample wettability. However, there is no pore-scale model to quantify this relationship.MethodsWe consider the simplest representation of a rock pore space: a bundle of capillary tubes of varying size. Equations describing mass and charge transfer through a single capillary are derived and the macroscopic zeta potential and wettability determined by integrating over capillaries. Model predictions are tested against measured data yielding a good match.FindingsMixed- and oil-wet models return a macro-scale zeta potential that is a combination of the micro-scale zeta potential of mineral-brine and oil-brine interfaces and the relationship between macro-scale zeta potential and water saturation exhibits hysteresis. The model predicts a similar relationship between zeta potential and wettability to that observed in experimental data but does not provide a perfect match. Fitting the model to experimental data allows the oil-brine zeta potential to be estimated at conditions where it cannot be measured directly. Results suggest that positive values of the oil-brine zeta potential may be more common than previously thought with implications for surface complexation models and the design of controlled salinity waterflooding of oil reservoirs.
Sparks RSJ, Blundy JD, Cashman K, et al., 2022, Large silicic magma bodies and very large magnitude explosive eruptions, BULLETIN OF VOLCANOLOGY, Vol: 84, ISSN: 0258-8900
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- Citations: 1
Al Kubaisy J, Salinas P, Jackson MD, 2022, Hybrid finite element pressure approximation for multiphase flow and transport in highly heterogeneous porous media
Control volume finite element (CVFE) methods are commonly used for modeling flow and transport in geometrically complex porous media domains with unstructured meshes. The CVFE approach is based on the finite element method to approximate the pressure and velocity fields, and uses the finite volume method to model saturation ensuring mass conservation. Control volumes are constructed by spanning element boundaries, leading to an artificial smearing of the numerical solution in the presence of sharp material interfaces. Recently, a CVFE method based on discontinuous pressure was introduced that enabled the construction of discontinuous control volumes, thus preventing control volumes from spanning element boundaries. This modification of the method provides accurate solutions but is computationally very expensive due to the discontinuous approximation which incorporates additional degrees of freedom per element. In this work, we propose using hybrid finite element pressure approximations to capture flow and transport in highly heterogeneous porous media. The CVFE element pair $P_{0,DG}-P_{1,H}$ denotes a constant, element-wise, discontinuous Galerkin velocity vector approximation and a hybrid (continuous/discontinuous) Galerkin first-order pressure scalar approximation of the flow model. The method exploits the efficient continuous CVFE method in most of the model domain while the discontinuous CVFE approach is applied exclusively along material discontinuities. We demonstrate that this hybrid scheme outperforms the classical CVFE continuous approach as well as the discontinuous Galerkin modification by incorporating the best of both approaches. The presented hybrid approach computational requirements are comparable to the continuous approach while the accuracy of the transport solution corresponds to that of the discontinuous pressure method. We validate the presented hybrid approach and discuss the convergence of the method. The effectiveness of the new scheme is de
Silva V, Regnier G, Salinas P, et al., 2022, Rapid modelling of reactive transport in porous media using machine learning
Reactive transport in porous media can play an important role in a variety of processes in subsurface reservoirs, such as groundwater flow, geothermal heat production, oil recovery and CO2 storage. However, numerical solution of fluid flow in porous media coupled with chemical reaction is very computationally demanding. Simultaneously, the success of machine learning in different fields has opened up new possibilities in reactive transport simulations. In this project, we focus on using machine learning techniques to replace the geochemical kinetic calculations generated by PHREEQC. PHREEQC is an open-source aqueous geochemical code that can be used in stand-alone mode or as a reaction module coupled with a flow and transport simulator. Here, we apply machine learning approaches to produce a fast proxy model of PHREEQC. This enables us to have a coupling between transport and reaction while minimizing the added computational cost. We focus initially on calcite dissolution during CO2 sequestration. Different machine learning techniques are investigated and compared to see which is more appropriate for the calcite dissolution problem. The proposed machine learning approach is designed to deal with different time-step sizes and unstructured elements. It accelerates the numerical simulation and proves to be practical to replace the reaction model presented in PHREEQC. This considerably reduces the computational cost of reactive transport while ensuring excellent simulation accuracy. The rapid modelling of reactive transport in porous media has a broad potential to replace many other phase equilibrium models across a wide range of reactive transport problems.
Alarouj M, Collini H, Jackson MD, 2021, Positive Zeta Potential in Sandstones Saturated With Natural Saline Brine, GEOPHYSICAL RESEARCH LETTERS, Vol: 48, ISSN: 0094-8276
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- Citations: 4
Kampitsis AE, Kostorz WJ, Muggeridge AH, et al., 2021, The life span and dynamics of immiscible viscous fingering in rectilinear displacements (vol 33, 096608, 2021), PHYSICS OF FLUIDS, Vol: 33, ISSN: 1070-6631
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- Citations: 1
Silva VLS, Salinas P, Jackson MD, et al., 2021, Machine learning acceleration for nonlinear solvers applied to multiphase porous media flow, Computer Methods in Applied Mechanics and Engineering, Vol: 384, Pages: 1-17, ISSN: 0045-7825
A machine learning approach to accelerate convergence of the nonlinear solver in multiphase flow problems is presented here. The approach dynamically controls an acceleration method based on numerical relaxation. It is demonstrated in a Picard iterative solver but is applicable to other types of nonlinear solvers. The aim of the machine learning acceleration is to reduce the computational cost of the nonlinear solver by adjusting to the complexity/physics of the system. Using dimensionless parameters to train and control the machine learning enables the use of a simple two-dimensional layered reservoir for training, while also exploring a wide range of the parameter space. Hence, the training process is simplified and it does not need to be rerun when the machine learning acceleration is applied to other reservoir models. We show that the method can significantly reduce the number of nonlinear iterations without compromising the simulation results, including models that are considerably more complex than the training case.
Titus Z, Heaney C, Jacquemyn C, et al., 2021, Conditioning surface-based geological models to well data using artificial neural networks, Computational Geosciences: modeling, simulation and data analysis, Vol: 26, Pages: 779-802, ISSN: 1420-0597
Surface-based modelling provides a computationally efficient approach for generating geometrically realistic representations of heterogeneity in reservoir models. However, conditioning Surface-Based Geological Models (SBGMs) to well data can be challenging because it is an ill-posed inverse problem with spatially distributed parameters. To aid fast and efficient conditioning, we use here SBGMs that model geometries using parametric, grid-free surfaces that require few parameters to represent even realistic geological architectures. A neural network is trained to learn the underlying process of generating SBGMs by learning the relationship between the parametrized SBGM inputs and the resulting facies identified at well locations. To condition the SBGM to these observed data, inverse modelling of the SBGM inputs is achieved by replacing the forward model with the pre-trained neural network and optimizing the network inputs using the back-propagation technique applied in training the neural network. An analysis of the uncertainties associated with the conditioned realisations demonstrates the applicability of the approach for evaluating spatial variations in geological heterogeneity away from control data in reservoir modelling. This approach for generating geologically plausible models that are calibrated with observed well data could also be extended to other geological modelling techniques such as object- and process-based modelling.
Kampitsis AE, Kostorz WJ, Muggeridge AH, et al., 2021, The life span and dynamics of immiscible viscous fingering in rectilinear displacements, PHYSICS OF FLUIDS, Vol: 33, ISSN: 1070-6631
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- Citations: 1
Salinas P, Regnier G, Jacquemyn C, et al., 2021, Dynamic mesh optimisation for geothermal reservoir modelling, Geothermics, Vol: 94, Pages: 1-13, ISSN: 0375-6505
Modelling geothermal reservoirs is challenging due to the large domain and wide range of length- and time-scales of interest. Attempting to represent all scales using a fixed computational mesh can be very computationally expensive. Application of dynamic mesh optimisation in other fields of computational fluid dynamics has revolutionised the accuracy and cost of numerical simulations. Here we present a new approach for modelling geothermal reservoirs based on unstructured meshes with dynamic mesh optimisation. The resolution of the mesh varies during a simulation, to minimize an error metric for solution fields of interest such as temperature and pressure. Efficient application of dynamic mesh optimisation in complex subsurface reservoirs requires a new approach to represent geologic heterogeneity and we use parametric spline surfaces to represent key geological features such as faults and lithology boundaries. The resulting 3D surface-based models are mesh free; a mesh is created only when required for numerical computations. Dynamic mesh optimisation preserves the surfaces and hence geologic heterogeneity. The governing equations are discretised using a double control volume finite element method that ensures heat and mass are conserved and provides robust solutions on distorted meshes. We apply the new method to a series of test cases that model sedimentary geothermal reservoirs. We demonstrate that dynamic mesh optimisation yields significant performance gains, reducing run times by up to 8 times whilst capturing flow and heat transport with the same accuracy as fixed meshes.
Lyu Z, Lei Q, Yang L, et al., 2021, A novel approach to optimising well trajectory in heterogeneous reservoirs based on the fast-marching method, Journal of Natural Gas Science and Engineering, Vol: 88, Pages: 1-12, ISSN: 1875-5100
To achieve efficient recovery of subsurface energy resources, a suitable trajectory needs to be identified for the production well. In this study, a new approach is presented for automated identification of optimum well trajectories in heterogeneous oil/gas reservoirs. The optimisation procedures are as follows. First, a productivity potential map is generated based on the site characterisation data of a reservoir (when available). Second, based on the fast-marching method, well paths are generated from a number of entrance positions to a number of exit points at opposite sides of the reservoir. The well trajectory is also locally constrained by a prescribed maximum curvature to ensure that the well trajectory is drillable. Finally, the optimum well trajectory is selected from all the candidate paths based on the calculation of a benefit-to-cost ratio. If required, a straight directional well path, may also be derived through a linear approximation to the optimised non-linear trajectory by least squares analysis. Model performance has been demonstrated in both 2D and 3D. In the 2D example, the benefit-to-cost ratio of the optimised well is much higher than that of a straight well; in the 3D example, laterals of various curvatures are generated. The applicability of the method is tested by exploring different reservoir heterogeneities and curvature constraints. This approach can be applied to determine the entrance/exit positions and the well path for subsurface energy system development, which is useful for field applications.
Jacquemyn C, Pataki MEH, Hampson GJ, et al., 2021, Sketch-based interface and modelling of stratigraphy and structure in three dimensions, Journal of the Geological Society, Vol: 178, Pages: 1-17, ISSN: 0016-7649
Geological modelling is widely used to predict resource potential in subsurface reservoirs. However, modelling is often slow, requires use of mathematical methods that are unfamiliar to many geoscientists, and is implemented in expert software. We demonstrate here an alternative approach using sketch-based interface and modelling, which allows rapid creation of complex three-dimensional (3D) models from 2D sketches. Sketches, either on vertical cross-sections or in map-view, are converted to 3D surfaces that outline geological interpretations. We propose a suite of geological operators that handle interactions between the surfaces to form a geologically realistic 3D model. These operators deliver the flexibility to sketch a geological model in any order and provide an intuitive framework for geoscientists to rapidly create 3D models. Two case studies are presented, demonstrating scenarios in which different approaches to model sketching are used depending on the geological setting and available data. These case studies show the strengths of sketching with geological operators. Sketched 3D models can be queried visually or quantitatively to provide insights into heterogeneity distribution, facies connectivity or dynamic model behaviour; this information cannot be obtained by sketching in 2D or on paper.
Kostorz WJ, Muggeridge AH, Jackson MD, 2021, Non-intrusive reduced order modeling: Geometrical framework, high-order models, and a priori analysis of applicability, INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN ENGINEERING, Vol: 122, Pages: 2545-2565, ISSN: 0029-5981
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- Citations: 2
Alarouj M, Ijioma A, Graham MT, et al., 2021, Numerical modelling of self-potential in subsurface reservoirs, Computers & Geosciences, Vol: 146, Pages: 1-19, ISSN: 0098-3004
We report a new, open-source, MATLAB-based 3D code for numerically simulating the self-potential (SP) in subsurface reservoirs. The code works as a post-processor, using outputs from existing reservoir flow and transport simulators at a selected timestep to calculate the SP throughout the reservoir model. The material properties required to calculate the SP are user defined and may be constant or vary in each cell. The code solves the equations governing flow and transport of electrical charge and global charge conservation using a control-volume-finite-difference scheme. Electrical currents associated with the SP may spread beyond the reservoir model domain, and the code allows for the domain to be extended vertically and laterally to account for this. Here, we present the governing equations and the numerical method used and demonstrate application of the code using an example in which we predict the SP signals associated with oil production from a subsurface reservoir supported by water injection.
Costa Sousa M, Silva J, Silva C, et al., 2020, Smart modelling of geologic stratigraphy concepts using sketches, Smart Tools and Applications in computer Graphics (STAG) 2020, Publisher: The Eurographics Association, Pages: 89-100
Several applications of Earth Science require geologically valid interpretation and visualization of complex physical structures in data-poor subsurface environments. Hand-drawn sketches and illustrations are standard practices used by domain experts for conceptualizing their observations and interpretations. These conceptual geo-sketches provide rich visual references for exploring uncertainties and helping users formulate ideas, suggest possible solutions, and make critical decisions affecting the various stages in geoscience studies and modelling workflows. In this paper, we present a sketch-based interfaces and modelling (SBIM) approach for the rapid conceptual construction of stratigraphic surfaces, which are common to most geologic modelling scales, studies, and workflows. Our SBIM approach mirrors the way domain users produce geo-sketches and uses them to construct 3D geologic models, enforcing algorithmic rules to ensure geologically-sound stratigraphic relationships are generated, and supporting different scales of geology being observed and interpreted. Results are presented for two case studies demonstrating the flexibility and broad applicability of our rule-based SBIM approach for conceptual stratigraphy.
Yekta A, Salinas P, Hajirezaie S, et al., 2020, Reactive transport modeling in heterogeneous porous media with dynamic mesh optimization, Computational Geosciences: modeling, simulation and data analysis, Vol: 25, Pages: 357-372, ISSN: 1420-0597
This paper presents a numerical simulator for solving compositional multiphase flow and reactive transport. The simulator was developed by effectively linking IC-FERST (Imperial College Finite Element Reservoir SimulaTor) with PHREEQCRM. IC-FERST is a next-generation three-dimensional reservoir simulator based on the double control volume finite element method and dynamic unstructured mesh optimization and is developed by the Imperial College London. PHREEQCRM is a state-of-the-art geochemical reaction package and is developed by the United States Geological Survey. We present a step-by-step framework on how the coupling is performed. The coupled code is called IC-FERST-REACT and is capable of simulating complex hydrogeological, biological, chemical, and mechanical processes occurring including processes occur during CO2 geological sequestration, CO2 enhanced oil recovery, and geothermal systems among others. In this paper, we present our preliminary work as well as examples related to CO2 geological sequestration. We performed the model coupling through developing an efficient application programming interface (API). IC-FERST-REACT inherits high-order methods and unstructured meshes with dynamic mesh optimization from IC-FERST. This reduces the computational cost by placing the mesh resolution where and when necessary and it can better capture flow instabilities if they occur. This can have a strong impact on reactive transport simulations which usually suffer from computational cost. From PHREEQCRM the code inherits the ability to efficiently model geochemical reactions. Benchmark examples are used to show the capability of IC-FERST-REACT in solving multiphase flow and reactive transport.
Li S, Jackson MD, Agenet N, 2020, Role of the calcite-water interface in wettability alteration during low salinity waterflooding, FUEL, Vol: 276, ISSN: 0016-2361
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- Citations: 12
Osman H, Graham GH, Moncorge A, et al., 2020, Is cell-to-cell scale variability necessary in reservoir models?, Mathematical Geosciences, Vol: 53, Pages: 271-296, ISSN: 1573-8868
Reservoir models typically contain hundreds-of-thousands to millions of grid cells in which petrophysical properties such as porosity and permeability vary on a cell-to-cell basis. However, although the petrophysical properties of rocks do vary on a point-to-point basis, this variability is not equivalent to the cell-to-cell variations in models. We investigate the impact of removing cell-to-cell variability on predictions of fluid flow in reservoir models. We remove cell-to-cell variability from models containing hundreds of thousands of unique porosity and permeability values to yield models containing just a few tens of unique porosity and permeability values grouped into a few internally homogeneous domains. The flow behavior of the original model is used as a reference. We find that the impact of cell-to-cell variability on predicted flow is small. Cell-to-cell variability is not necessary to capture flow in reservoir models; rather, it is the spatially correlated variability in petrophysical properties that is important. Reservoir modelling effort should focus on capturing correlated geologic domains in the most realistic and computationally efficient manner.
Kostorz WJ, Muggeridge AH, Jackson MD, 2020, An efficient and robust method for parameterized nonintrusive reduced-order modeling, INTERNATIONAL JOURNAL FOR NUMERICAL METHODS IN ENGINEERING, Vol: 121, Pages: 4674-4688, ISSN: 0029-5981
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- Citations: 6
Lei Q, Jackson MD, Muggeridge AH, et al., 2020, Modelling the reservoir-to-tubing pressure drop imposed by multiple autonomous inflow control devices installed in a single completion joint in a horizontal well, Journal of Petroleum Science and Engineering, Vol: 189, Pages: 1-16, ISSN: 0920-4105
Autonomous inflow control devices (AICDs) are used to introduce an additional pressure drop between the reservoir and the tubing of a production well that depends on the fluid phase flowing into the device: a larger pressure drop is introduced when unwanted phases such as water or gas enter the AICD. The additional pressure drop is typically represented in reservoir simulation models using empirical relationships fitted to experimental data for a single AICD. This approach may not be correct if each completion joint is equipped with multiple AICDs as the flow at different AICDs may be different. We use high-resolution numerical modelling to determine the total additional pressure drop introduced by two AICDs installed in a single completion joint in a horizontal well. The model captures the multiphase flow of oil and water through the inner annulus into each AICD. We explore a number of relevant oil-water inflow scenarios with different flow rates and water cuts. Our results show that if only one AICD is installed, the additional pressure drop is consistent with the experimentalzly-derived empirical formulation. However, if two AICDs are present, there is a significant discrepancy between the additional pressure drop predicted by the simulator and the empirical relationship. This discrepancy occurs because each AICD has a different total and individual phase flow rate, and the final steady-state flow results from a self-organising mechanism emerging from the system. We report the discrepancy as a water cut-dependent correction to the empirical equation, which can be used in reservoir simulation models to better capture the pressure drop across a single completion containing two AICDs. Our findings highlight the importance of understanding how AICDs modify flow into production wells, and have important consequences for improving the representation of advanced wells in reservoir simulation models.
Zhang Z, Geiger S, Rood M, et al., 2020, Fast flow computation methods on unstructured tetrahedral meshes for rapid reservoir modelling, Computational Geosciences, Vol: 24, Pages: 641-661, ISSN: 1420-0597
Subsurface reservoir models have a high degree of uncertainty regarding reservoir geometry and structure. A range of conceptual models should therefore be generated to explore how fluids-in-place, reservoir dynamics, and development decisions are affected by such uncertainty. The rapid reservoir modelling (RRM) workflow has been developed to prototype reservoir models across scales and test their dynamic behaviour. RRM complements existing workflows in that conceptual models can be prototyped, explored, compared, and ranked rapidly prior to detailed reservoir modelling. Reservoir geology is sketched in 2D with geological operators and translated in real-time into geologically correct 3D models. Flow diagnostics provide quantitative information for these reservoir model prototypes about their static and dynamic behaviours. A tracing algorithm is reviewed and implemented to compute time-of-flight and tracer concentrations efficiently on unstructured grids. Numerical well testing (NWT) is adopted in RRM to further interrogate the reservoir model. A new edge-based fast marching method is developed and implemented to solve the diffusive time-of-flight for approximating pressure transients efficiently on unstructured tetrahedral meshes. We demonstrate that an implementation of the workflow consisting of integrated sketch-based interface modelling, unstructured mesh generation, flow diagnostics, and numerical well testing is possible.
Collini H, Li S, Jackson MD, et al., 2020, Zeta potential in intact carbonates at reservoir conditions and its impact on oil recovery during controlled salinity waterflooding, Fuel, Vol: 266, Pages: 1-16, ISSN: 0016-2361
It is well known that oil recovery from carbonate reservoirs can be increased by modifying the injected brine composition in a process ‘controlled salinity water-flooding’ (CSW). However, the mineral- to pore- scale processes responsible for improved oil recovery (IOR) during CSW remain ambiguous and there is no method to predict the optimum CSW composition for a given crude-oil-brine rock system. Here we report the first integrated experimental measurements of zeta potential and IOR during CSW obtained at reservoir conditions. The zeta potential is a measure of the electrical potential at mineral-brine and oil-brine interfaces and controls the electrostatic forces acting between these interfaces.We find that the measured zeta potential in clean samples saturated with formation brine is typically positive and becomes more negative with brine dilution irrespective of temperature. After aging and wettability alteration, the zeta potential changes and we suggest a more positive zeta potential indicates a positive zeta potential at the oil-brine interface and vice-versa. Injecting low salinity brine yields IOR when the oil-brine zeta potential is identified to be negative, but no response when it is identified to be positive, consistent with the hypothesis that IOR during CSW is caused by an increase in the repulsive electrostatic force acting between mineral-brine and oil-brine interfaces. We suggest that the optimum brine composition for IOR during CSW should be chosen to yield the largest change in zeta potential at the mineral-brine interface with opposing polarity to the oil-brine interface and can be determined using the experimental method reported here.
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