Imperial College London

Dr Marc Stettler

Faculty of EngineeringDepartment of Civil and Environmental Engineering

Senior Lecturer
 
 
 
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Contact

 

+44 (0)20 7594 2094m.stettler Website

 
 
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Location

 

614Skempton BuildingSouth Kensington Campus

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Summary

 

Publications

Publication Type
Year
to

28 results found

Yang L, Zhang L, Stettler MEJ, Sukitpaneenit M, Xiao D, van Dam KHet al., 2020, Supporting an integrated transportation infrastructure and public space design: A coupled simulation method for evaluating traffic pollution and microclimate, Sustainable Cities and Society, Vol: 52, ISSN: 2210-6707

Traditional urban and transport infrastructure planning that emphasized motorized transport has fractured public space systems and worsened environmental quality, leading to a decrease in active travel. A novel multiscale simulation method for supporting an integrated transportation infrastructure and public space design is presented in this paper. This method couples a mesoscale agent-based traffic prediction model, traffic-related emission calculation, microclimate simulations, and human thermal comfort assessment. In addition, the effects of five urban design strategies on traffic pollution and pedestrian level microclimate are evaluated (i.e., a “two-fold” evaluation). A case study in Beijing, China, is presented utilizing the proposed urban modeling-design framework to support the assessment of a series of transport infrastructure and public space scenarios, including the Baseline scenario, a System-Internal Integration scenario, and two External Integration scenarios. The results indicate that the most effective way of achieving an environmentally- and pedestrian- friendly urban design is to concentrate on both the integration within the transport infrastructure and public space system and the mitigation of the system externalities (e.g., air pollution and heat exhaustion). It also demonstrates that the integrated blue-green approach is a promising way of improving local air quality, micro-climatic conditions, and human comfort.

Journal article

Brito TLF, Islam T, Stettler M, Mouette D, Meade N, Moutinho dos Santos Eet al., 2019, Transitions between technological generations of alternative fuel vehicles in Brazil, Energy Policy, Vol: 134, Pages: 110915-110915, ISSN: 0301-4215

The transportation sector is responsible for nearly a quarter of greenhouse gases emissions (GHG); thus, incisive policies are necessary to mitigate the sector’s effect on climate change. Promoting alternative fuel vehicles (AFV) is an essential strategy to reduce GHG emissions in the short term. Here, we study the effects of governmental incentives on the diffusion of ethanol and flex-fuel vehicle technologies in Brazil. We use a multi-generation diffusion model which assumes that new technologies introduce fresh market potential for adopters as well as upgraders from established technologies. Our analysis indicates that tax rates affected the adoption of both gasoline and ethanol technology, but for flex vehicles, the effect of taxation is not significant. The effect of fuel price shocks during the 1990s meant that the introduction of ethanol technology made no significant impact on market potential and a negative word-of-mouth effect contributed to the technology’s failure. In contrast, the introduction of flex technology led to almost a doubling of total market potential. As policy suggestions, we emphasise the importance of tax reduction in addition to promoting versatile technologies, which insulate consumers against price fluctuations.

Journal article

Woodward H, Stettler M, Pavlidis D, Aristodemou E, ApSimon H, Pain Cet al., 2019, A large eddy simulation of the dispersion of traffic emissions by moving vehicles at an intersection, Atmospheric Environment, Vol: 215, Pages: 1-16, ISSN: 1352-2310

Traffic induced flow within urban areas can have a significant effect on pollution dispersion, particularly for traffic emissions. Traffic movement results in increased turbulence within the street and the dispersion of pollutants by vehicles as they move through the street. In order to accurately model urban air quality and perform meaningful exposure analysis at the microscale, these effects cannot be ignored. In this paper we introduce a method to simulate traffic induced dispersion at high resolution. The computational fluid dynamics software, Fluidity, is used to model the moving vehicles through a domain consisting of an idealised intersection. A multi-fluid method is used where vehicles are represented as a second fluid which displaces the air as it moves through the domain. The vehicle model is coupled with an instantaneous emissions model which calculates the emission rate of each vehicle at each time step. A comparison is made with a second Fluidity model which simulates the traffic emissions as a line source and does not include moving vehicles. The method is used to demonstrate how moving vehicles can have a significant effect on street level concentration fields and how large vehicles such as buses can also cause acute high concentration events at the roadside which can contribute significantly to overall exposure.

Journal article

Grylls T, Le Cornec CMA, Salizzoni P, Soulhac L, Stettler MEJ, Van Reeuwijk Met al., Evaluation of an operational air quality model using large-eddy simulation, Atmospheric Environment: X, Vol: 3, ISSN: 2590-1621

The large-eddy simulation (LES) model uDALES is used to evaluate the predictive skill of the operational air quality model SIRANE. The use of LES in this study presents a novel approach to air quality model evaluation, avoiding sources of uncertainty and providing numerical control that permits systematic analysis of targeted parametrisations and assumptions.A case study is conducted over South Kensington, London with the morphology, emissions, meteorological conditions and boundary conditions carefully matched in both models. The dispersion of both inert (NOx) and reactive (NO, NO2 and O3) pollutants under neutral, steady-state conditions is simulated for a south-westerly and westerly wind direction. A quantitative comparison between the two models is performed using statistical indices (the fractional bias, FB, the normalised mean squared error, NMSE, and the fraction in a factor of 2, FAC2).SIRANE is shown to successfully capture the dominant trends with respect to canyon-averaged concentrations of inert NOx (FB = -0.08, NMSE = 0.08 and FAC2 = 1.0). The prediction of along-canyon velocities is shown to exhibit sources of systematic error dependant on the angle of incidence of the mean wind (FB = -0.18). The assumption of photostationarity within SIRANE (deviations from equilibrium of up to 170% exist close to busy roads) is also identified as a significant source of systematic bias resulting in over- and underpredictions of NO2 (FB = -0.18) and O3 (FB = 0.14) respectively. The validity of the assumed uniform in-canyon concentration is assessed by analysing the pedestrian, leeward and windward concentrations resolved in uDALES. The use of canyon-averaged concentrations to predict pedestrian level exposure is shown to result in significant underestimations. Linear regression is used to effectively capture the relationship between pedestrian- and canyon-averaged concentrations in uDALES. Correction factors are derived (m ≈ 1.62 and R 2 = 0.92 for inert NOx) th

Journal article

Teoh R, Stettler MEJ, Majumdar A, Schumann U, Graves B, Boies AMet al., 2019, A methodology to relate black carbon particle number and mass emissions, Journal of Aerosol Science, Vol: 132, Pages: 44-59, ISSN: 0021-8502

Black carbon (BC) particle number (PN) emissions from various sources contribute to the deterioration of air quality, adverse health effects, and anthropogenic climate change. This paper critically reviews different fractal aggregate theories to develop a new methodology that relates BC PN and mass concentrations (or emissions factors). The new methodology, named as the fractal aggregate (FA) model is validated with measurements from three different BC emission sources: an internal combustion engine, a soot generator, and two aircraft gas turbine engines at ground and cruise conditions. Validation results of the FA model show that R 2 values range from 0.44 to 0.95, while the Normalised Mean Bias is between −27.7% and +26.6%. The model estimates for aircraft gas turbines represent a significant improvement compared to previous methodologies used to estimate aviation BC PN emissions, which relied on simplified assumptions. Uncertainty and sensitivity analyses show that the FA model estimates have an asymmetrical uncertainty bound (−54%,+103%) at a 95% confidence interval for aircraft gas turbine engines and are most sensitive to uncertainties in the geometric standard deviation of the BC particle size distribution. Given the improved performance in estimating BC PN emissions from various sources, we recommend the implementation of the FA model in future health and climate assessments, where the impacts of PN are significant.

Journal article

Achurra-Gonzalez PE, Angeloudis P, Goldbeck N, Graham D, Zavitsas K, Stettler Met al., Evaluation of port disruption impacts in the global liner shipping network, Journal of Shipping and Trade, ISSN: 2364-4575

The global container shipping network is vital to international trade. Current techniques for its vulnerability assessment are constrained due to the lack of historical disruption data and computational limitations due to typical network sizes. We address these modelling challenges by developing a new framework, composed by a game-theoretic attacker-defender model and a cost-based container assignment model that can identify systemic vulnerabilities in the network. Given its focus on logic and structure, the proposed framework has minimal input data requirements and does not rely on the presence of extensive historical disruption data. Numerical implementations are carried in a global-scale liner network where disruptions occur in Europe’s main container ports. Model outputs are used to establish performance baselines for the network and illus-trate the differences in regional vulnerability levels and port criticality rankings with different disruption magnitudes and flow diversion strategies. Sensitivity analysis of these outputs identifies network compo-nents that are more susceptible to lower levels of disruption which are more common in practice and to assess the effectiveness of component-level interventions seeking to increase the resilience of the system.

Journal article

Speirs J, Balcombe P, Blomerus P, Stettler M, Brandon N, Hawkes Aet al., 2019, Can natural gas reduce emissions from transport?: Heavy goods vehicles and shipping

Report

Karamanis R, Angeloudis P, Sivakumar A, Stettler Met al., 2018, Dynamic Pricing in One-Sided Autonomous Ride-Sourcing Markets, 21st IEEE International Conference on Intelligent Transportation Systems (ITSC), Publisher: IEEE, Pages: 3645-3650, ISSN: 2153-0009

Conference paper

Koudis GS, Hu SJ, Majumdar A, Ochieng WY, Stettler MEJet al., 2018, The impact of single engine taxiing on aircraft fuel consumption and pollutant emissions, Aeronautical Journal, Vol: 122, Pages: 1967-1984, ISSN: 0001-9240

Optimisation of aircraft ground operations to reduce airport emissions can reduce resultant local air quality impacts. Single engine taxiing (SET), where only half of the installed number of engines are used for the majority of the taxi duration, offers the opportunity to reduce fuel consumption, and emissions of NOX, CO and HC. Using 3510 flight data records, this paper develops a model for SET operations and presents a case study of London Heathrow, where we show that SET is regularly implemented during taxi-in. The model predicts fuel consumption and pollutant emissions with greater accuracy than previous studies that used simplistic assumptions. Without SET during taxi-in, fuel consumption and pollutant emissions would increase by up to 50%. Reducing the time before SET is initiated to the 25th percentile of recorded values would reduce fuel consumption and pollutant emissions by 7–14%, respectively, relative to current operations. Future research should investigate the practicalities of reducing the time before SET initialisation so that additional benefits of reduced fuel loadings, which would decrease fuel consumption across the whole flight, can be achieved.

Journal article

Popoola OAM, Carruthers D, Lad C, Bright VB, Mead M, Stettler MEJ, Saffell JR, Jons RLet al., 2018, Use of networks of low cost air quality sensors to quantify air quality in urban settings, Atmospheric Environment, Vol: 194, Pages: 58-70, ISSN: 1352-2310

Low cost sensors are becoming increasingly available for studying urban air quality. Here we show how such sensors, deployed as a network, provide unprecedented insights into the patterns of pollutant emissions, in this case at London Heathrow Airport (LHR). Measurements from the sensor network were used to unequivocally distinguish airport emissions from long range transport, and then to infer emission indices from the various airport activities. These were used to constrain an air quality model (ADMS-Airport), creating a powerful predictive tool for modelling pollutant concentrations. For nitrogen dioxide (NO2), the results show that the non-airport component is the dominant fraction (∼75%) of annual NO2 around the airport and that despite a predicted increase in airport related NO2 with an additional runway, improvements in road traffic fleet emissions are likely to more than offset this increase. This work focusses on London Heathrow Airport, but the sensor network approach we demonstrate has general applicability for a wide range of environmental monitoring studies and air pollution interventions.

Journal article

Ainalis D, Achurra-Gonzalez P, Gaudin A, Garcia de la Cruz JM, Angeloudis P, Ochieng WY, Stettler MEJet al., Ultra-Capacitor based kinetic energy recovery system for heavy goods vheicles, 15th International Symposium on Heavy Vehicle Transport Technology

The Climate Change Act 2008 commits the UK to reduce the Greenhouse Gas emissions by 80% by 2050 relative to 1990 levels. While Heavy Goods Vehicles and buses contribute about 4% of the total Greenhouse Gas emissions in the UK, these emissions only decrease by 10% between 1990 and 2015. Urban areas are particularly susceptible to emissions and can have a significant impact upon the health of residents. For Heavy Goods Vehicles, braking losses are one of the most significant losses. A Kinetic Energy Recovery System can help reduce these emissions, and increase fuel efficiency by up to 30 %. This paper describes an InnovateUK funded project aimed at evaluating the technical and economic feasibility of a retrofitted Kinetic Energy Recovery System on Heavy Goods Vehicles through an operational trial, controlled emissions and fuel tests, and numerical modelling. A series of preliminary results using a numerical vehicle model is compared with operational data, along with simulations comparing the fuel efficiency of a Heavy Goods Vehicle with and without the KERS.

Conference paper

Karamanis R, Angeloudis P, Sivakumar A, Stettler Met al., Market dynamics between public transport and competitive ride-sourcing providers, 7th Symposium of the European Association for Research in Transportation, Publisher: hEART

Conference paper

O'Driscoll R, Stettler MEJ, Molden N, Oxley T, ApSimon HMet al., 2017, Real world CO2 and NOx emissions from 149 Euro 5 and 6 diesel, gasoline and hybrid passenger cars., Science of the Total Environment, Vol: 621, Pages: 282-290, ISSN: 0048-9697

In this study CO2 and NOx emissions from 149 Euro 5 and 6 diesel, gasoline and hybrid passenger cars were compared using a Portable Emissions Measurement System (PEMS). The models sampled accounted for 56% of all passenger cars sold in Europe in 2016. We found gasoline vehicles had CO2 emissions 13-66% higher than diesel. During urban driving, the average CO2 emission factor was 210.5 (sd. 47) gkm-1 for gasoline and 170.2 (sd. 34) gkm-1 for diesel. Half the gasoline vehicles tested were Gasoline Direct Injection (GDI). Euro 6 GDI engines <1.4ℓ delivered ~17% CO2 reduction compared to Port Fuel Injection (PFI). Gasoline vehicles delivered an 86-96% reduction in NOx emissions compared to diesel cars. The average urban NOx emission from Euro 6 diesel vehicles 0.44 (sd. 0.44) gkm-1 was 11 times higher than for gasoline 0.04 (sd. 0.04) gkm-1. We also analysed two gasoline-electric hybrids which out-performed both gasoline and diesel for NOx and CO2. We conclude action is required to mitigate the public health risk created by excessive NOx emissions from modern diesel vehicles. Replacing diesel with gasoline would incur a substantial CO2 penalty, however greater uptake of hybrid vehicles would likely reduce both CO2 and NOx emissions. Discrimination of vehicles on the basis of Euro standard is arbitrary and incentives should promote vehicles with the lowest real-world emissions of both NOx and CO2.

Journal article

Koudis GS, Hu SJ, North RJ, Majumdar A, Stettler MEJet al., 2017, The impact of aircraft takeoff thrust setting on NO<inf>X</inf> emissions, Journal of Air Transport Management, Vol: 65, Pages: 191-197, ISSN: 0969-6997

Reduced thrust takeoff has the potential to reduce aircraft-related NO X emissions at airports, however this remains to be investigated using flight data. This paper analyses the effect of takeoff roll thrust setting variability on the magnitude and spatial distribution of NO X emissions using high-resolution data records for 497 Airbus A319 activities at London Heathrow. Thrust setting varies between 67 and 97% of maximum, and aircraft operating in the bottom 10th percentile emit on average 514 g less NO X per takeoff roll (32% reduction) than the top 10th percentile, however this is dependent on takeoff roll duration. Spatial analysis suggests that peak NO X emissions, corresponding to the start of the takeoff roll, can be reduced by up to 25% by adopting reduced thrust takeoff activities. Furthermore, the length of the emission source also decreases. Consequently, the use of reduced thrust takeoff may enable improved local air quality at airports.

Journal article

Koudis GS, Hu J, Majumdar A, Jones R, Stettler MEJet al., 2017, Airport emissions reductions from reduced thrust takeoff operations, Transportation Research Part D: Transport and Environment, Vol: 52, Pages: 15-28, ISSN: 1879-2340

Given forecast aviation growth, many airports are predicted to reach capacity and require expansion. However, pressure to meet air quality regulations emphasises the importance of efficient ground-level aircraft activities to facilitate growth. Operational strategies such as reducing engine thrust setting at takeoff can reduce fuel consumption and pollutant emissions; however, quantification of the benefits and consistency of its use have been limited by data restrictions. Using 3,336 high-resolution flight data records, this paper analyses the impact of reduced thrust takeoff at London Heathrow. Results indicate that using reduced thrust takeoff reduces fuel consumption, nitrogen oxides (NOX) and black carbon (BC) emissions by 1.0-23.2%, 10.7-47.7%, and 49.0-71.7% respectively, depending on aircraft-engine combinations relative to 100% thrust takeoff. Variability in thrust settings for the same aircraft-engine combination and dependence on takeoff weight (TOW) is quantified. Consequently, aircraft-engine specific optimum takeoff thrust settings that minimise fuel consumption and pollutant emissions for different aircraft TOWs are presented. Further reductions of 1.9%, 5.8% and 6.5% for fuel consumption, NOX and BC emissions could be achieved, equating to reductions of approximately 0.4%, 3.5% and 3.3% in total ground level fuel consumption, NOX and BC emissions. These results quantify the contribution that reduced thrust operations offer towards achieving industry environmental targets and air quality compliance, and imply that the current implementation of reduced thrust takeoff at Heathrow is near optimal, considering operational and safety constraints.

Journal article

Olfert JS, Dickau M, Momenimovahed A, Saffaripour M, Thompson K, Smallwood G, Stettler MEJ, Boies AM, Sevcenco Y, Crayford A, Johnson Met al., 2017, Effective density and volatility of particles sampled from a helicopter gas turbine engine, Aerosol Science and Technology, Vol: 51, Pages: 704-714, ISSN: 0278-6826

The effective density and size-resolved volatility of particles emitted from a Rolls-Royce Gnome helicopter turboshaft engine are measured at two engine speed settings (13,000 and 22,000 RPM). The effective density of denuded and undenuded particles were measured. The denuded effective densities are similar to the effective densities of particles from a gas turbine with a double annular combustor as well as a wide variety of internal combustion engines. The denuded effective density measurements were also used to estimate the size and number of primary particles in the soot aggregates. The primary particle size estimates show that the primary particle size was smaller at lower engine speed (in agreement with transmission electron microscopy analysis). As a demonstration, the size-resolved volatility of particles emitted from the engine are measured with a system consisting of a differential mobility analyzer, centrifugal particle mass analyzer, condensation particle counter, and catalytic stripper. This system determines the number distributions of particles that contain or do not contain non-volatile material, and the mass distributions of non-volatile material, volatile material condensed onto the surface of non-volatile particles, and volatile material forming independent particles (e.g. nucleated volatile material). It was found that the particulate at 13,000 RPM contained a measurable fraction of purely volatile material with diameters below ∼25 nm and had a higher mass fraction of volatile material condensed on the surface of the soot (6–12%) compared to the 22,000 RPM condition (1–5%). This study demonstrates the potential to quantify the distribution of volatile particulate matter and gives additional information to characterize sampling effects with regulatory measurement procedures.

Journal article

Worth DJ, Stettler MEJ, Dickinson P, Hegarty K, Boies AMet al., 2016, Characterization and evaluation of methane oxidation catalysts for dual-fuel diesel and natural gas engines, Emission Control Science and Technology, Vol: 2, Pages: 204-214, ISSN: 2199-3629

The UK has incentivized the use of natural gas in heavy goods vehicles (HGVs) by converting to dual-fuel (DF) diesel-natural gas systems to reduce noxious and greenhouse gas emissions. Laboratory and on-road measurements of DF vehicles have demonstrated a decrease in CO2 emissions relative to diesel, but there is an increase in greenhouse gas (CO2e) emissions because of unburned methane. Decreasing tailpipe emissions of methane via after-treatment devices in lean-burn compression ignition engines is a challenge because of low exhaust temperatures (∼400 °C) and the presence of water vapor. In this study, six commercially available methane oxidation catalysts (MOCs) were tested for their application in DF HGV vehicles. Each MOC was characterized in terms of the catalyst platinum group metal (PGM) loading (both Pd and Pt), particle size, catalytic surface area, and Pd:Pt ratio. In addition, the washcoat surface area, pore volume, and pore size were evaluated. The MOC conversion efficiency was evaluated in controlled methane-oxidation experiments with varying temperatures, flow rates, and gas compositions. Characteristic-conversion efficiency correlations demonstrate that the influential MOC characteristics were PGM loading (both Pd and Pt), Pd:Pt ratio, washcoat surface area, and washcoat pore volume. With 90 % methane oxidation at less than 400 °C in DF HGV exhaust conditions, sample 1 had the highest conversion efficiency because of a high PGM loading (330 g/ft3, 12,000 g/m3), a 5.9 Pd:Pt ratio, a high alumina washcoat surface area of 20 m2/cm3, and 74-mm3/cm3 pore volume. Additional studies showed increased MOC conversion efficiency with decreasing gas hourly space velocities (GHSVs) and increasing methane concentrations.

Journal article

O'Driscoll R, ApSimon HM, Oxley T, Molden N, Stettler MEJ, Thiyagarajah Aet al., 2016, A Portable Emissions Measurement System (PEMS) study of NO<inf>x</inf> and primary NO<inf>2</inf> emissions from Euro 6 diesel passenger cars and comparison with COPERT emission factors, Atmospheric Environment, Vol: 145, Pages: 81-91, ISSN: 1352-2310

© 2016 Elsevier Ltd Real world emissions of oxides of nitrogen (NOx) often greatly exceed those achieved in the laboratory based type approval process. In this paper the real world emissions from a substantial sample of the latest Euro 6 diesel passenger cars are presented with a focus on NOx and primary NO2. Portable Emissions Measurement System (PEMS) data is analysed from 39 Euro 6 diesel passenger cars over a test route comprised of urban and motorway sections. The sample includes vehicles installed with exhaust gas recirculation (EGR), lean NOx traps (LNT), or selective catalytic reduction (SCR). The results show wide variability in NOx emissions from 1 to 22 times the type approval limit. The average NOx emission, 0.36 (sd. 0.36) g km−1, is 4.5 times the Euro 6 limit. The average fraction primary NO2 (fNO2) is 44 (sd. 20) %. Higher emissions during the urban section of the route are attributed to an increased number of acceleration events. Comparisons between PEMS measurements and COPERT speed dependent emissions factors show PEMS measurements to be on average 1.6 times higher than COPERT estimates for NOx and 2.5 times for NO2. However, by removing the 5 most polluting vehicles average emissions were reduced considerably.

Journal article

Bishop JDK, Stettler MEJ, Molden N, Boies AMet al., 2016, Engine maps of fuel use and emissions from transient driving cycles, Applied Energy, Vol: 183, Pages: 202-217, ISSN: 0306-2619

Air pollution problems persist in many cities throughout the world, despite drastic reductions in regulated emissions of criteria pollutants from vehicles when tested on standardised driving cycles. New vehicle emissions regulations in the European Union and United States require the use of OBD and portable emissions measurement systems (PEMS) to confirm vehicles meet specified limits during on-road operation. The resultant in-use testing will yield a large amount of OBD and PEMS data across a range of vehicles. If used properly, the availability of OBD and PEMS data could enable greater insight into the nature of real-world emissions and allow detailed modelling of vehicle energy use and emissions. This paper presents a methodology to use this data to create engine maps of fuel use and emissions of nitrous oxides (NOx), carbon dioxide (CO2) and carbon monoxide (CO). Effective gear ratios, gearbox shift envelopes, candidate engine maps and a set of vehicle configurations are simulated over driving cycles using the ADVISOR powertrain simulation tool. This method is demonstrated on three vehicles – one truck and two passenger cars – tested on a vehicle dynamometer and one driven with a PEMS. The optimum vehicle configuration and associated maps were able to reproduce the shape and magnitude of observed fuel use and emissions on a per second basis. In general, total simulated fuel use and emissions were within 5% of observed values across the three test cases. The fitness of this method for other purposes was demonstrated by creating cold start maps and isolating the performance of tailpipe emissions reduction technologies. The potential of this work extends beyond the creation of vehicle engine maps to allow investigations into: emissions hot spots; real-world emissions factors; and accurate air quality modelling using simulated per second emissions from vehicles operating in over any driving cycle.

Journal article

Dickau M, Olfert J, Stettler MEJ, Boies A, Momenimovahed A, Thomson K, Smallwood G, Johnson Met al., 2016, Methodology for quantifying the volatile mixing state of an aerosol, Aerosol Science and Technology, Vol: 50, Pages: 759-772, ISSN: 0278-6826

Mixing state refers to the relative proportions of chemical species in an aerosol, and the way these species are combined; either as a population where each particle consists of a single species (‘externally mixed’) or where all particles individually consist of two or more species (‘internally mixed’) or the case where some particles are pure and some particles consist of multiple species. The mixing state affects optical and hygroscopic properties, and quantifying it is therefore important for studying an aerosol's climate impact. In this article, we describe a method to quantify the volatile mixing state of an aerosol using a differential mobility analyzer, centrifugal particle mass analyzer, catalytic denuder, and condensation particle counter by measuring the mass distributions of the volatile and non-volatile components of an aerosol and determining how the material is mixed within and between particles as a function of mobility diameter. The method is demonstrated using two aerosol samples from a miniCAST soot generator, one with a high elemental carbon (EC) content, and one with a high organic carbon (OC) content. The measurements are presented in terms of the mass distribution of the volatile and non-volatile material, as well as measures of diversity and mixing state parameter. It was found that the high-EC soot nearly consisted of only pure particles where 86% of the total mass was non-volatile. The high-OC soot consisted of either pure volatile particles or particles that contained a mixture of volatile and non-volatile material where 8% of the total mass was pure volatile particles and 70% was non-volatile material (with the remaining 22% being volatile material condensed on non-volatile particles). © 2016 American Association for Aerosol Research

Journal article

Stettler MEJ, Midgley WJB, Swanson JJ, Cebon D, Boies AMet al., 2016, Greenhouse gas and noxious emissions from dual fuel diesel and natural gas heavy goods vehicles, Environmental Science & Technology, Vol: 50, Pages: 2018-2026, ISSN: 0013-936X

Dual fuel diesel and natural gas heavy goods vehicles (HGVs) operate on a combination of the two fuels simultaneously. By substituting diesel for natural gas, vehicle operators can benefit from reduced fuel costs and as natural gas has a lower CO2 intensity compared to diesel, dual fuel HGVs have the potential to reduce greenhouse gas (GHG) emissions from the freight sector. In this study, energy consumption, greenhouse gas and noxious emissions for five after-market dual fuel configurations of two vehicle platforms are compared relative to their diesel-only baseline values over transient and steady state testing. Over a transient cycle, CO2 emissions are reduced by up to 9%; however, methane (CH4) emissions due to incomplete combustion lead to CO2e emissions that are 50–127% higher than the equivalent diesel vehicle. Oxidation catalysts evaluated on the vehicles at steady state reduced CH4 emissions by at most 15% at exhaust gas temperatures representative of transient conditions. This study highlights that control of CH4 emissions and improved control of in-cylinder CH4 combustion are required to reduce total GHG emissions of dual fuel HGVs relative to diesel vehicles.

Journal article

Boies AM, Stettler MEJ, Swanson JJ, Johnson TJ, Olfert JS, Johnson M, Eggersdorfer ML, Rindlisbacher T, Wang J, Thomson K, Smallwood G, Sevcenco Y, Walters D, Williams PI, Corbin J, Mensah AA, Symonds J, Dastanpour R, Rogak SNet al., 2015, Particle Emission Characteristics of a Gas Turbine with a Double Annular Combustor, AEROSOL SCIENCE AND TECHNOLOGY, Vol: 49, Pages: 842-855, ISSN: 0278-6826

Journal article

Omu A, Rysanek A, Stettler M, Choudhary Ret al., 2015, Economic, Climate Change, and Air Quality Analysis of Distributed Energy Resource Systems, INTERNATIONAL CONFERENCE ON COMPUTATIONAL SCIENCE, ICCS 2015 COMPUTATIONAL SCIENCE AT THE GATES OF NATURE, Vol: 51, Pages: 2147-2156, ISSN: 1877-0509

Journal article

Simone NW, Stettler MEJ, Barrett SRH, 2013, Rapid estimation of global civil aviation emissions with uncertainty quantification, TRANSPORTATION RESEARCH PART D-TRANSPORT AND ENVIRONMENT, Vol: 25, Pages: 33-41, ISSN: 1361-9209

Journal article

Stettler MEJ, Swanson JJ, Barrett SRH, Boies AMet al., 2013, Updated Correlation Between Aircraft Smoke Number and Black Carbon Concentration, AEROSOL SCIENCE AND TECHNOLOGY, Vol: 47, Pages: 1205-1214, ISSN: 0278-6826

Journal article

Stettler MEJ, Boies AM, Petzold A, Barrett SRHet al., 2013, Global Civil Aviation Black Carbon Emissions, ENVIRONMENTAL SCIENCE & TECHNOLOGY, Vol: 47, Pages: 10397-10404, ISSN: 0013-936X

Journal article

Yim SHL, Stettler MEJ, Barrett SRH, 2013, Air quality and public health impacts of UK airports. Part II: Impacts and policy assessment, ATMOSPHERIC ENVIRONMENT, Vol: 67, Pages: 184-192, ISSN: 1352-2310

Journal article

Stettler MEJ, Eastham S, Barrett SRH, 2011, Air quality and public health impacts of UK airports. Part I: Emissions, ATMOSPHERIC ENVIRONMENT, Vol: 45, Pages: 5415-5424, ISSN: 1352-2310

Journal article

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