Imperial College London
Alternate

Professor Nilay Shah OBE FREng

Faculty of Engineering, Department of Chemical Engineering

Professor of Process Systems Engineering
 
 
 
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Contact

 

+44 (0)20 7594 6621n.shah

 
 
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Assistant

 

Miss Jessica Baldock +44 (0)20 7594 5699

 
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Location

 

ACEX 522ACE ExtensionSouth Kensington Campus

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Summary

 

Publications

Citation

BibTex format

@article{Baharudin:2022:10.1016/j.jcou.2022.102050,
author = {Baharudin, L and Rahmat, N and Othman, NH and Shah, N and Syed-Hassan, SSA},
doi = {10.1016/j.jcou.2022.102050},
journal = {Journal of CO2 Utilization},
title = {Formation, control, and elimination of carbon on Ni-based catalyst during CO<inf>2</inf>and CH<inf>4</inf>conversion via dry reforming process: A review},
url = {http://dx.doi.org/10.1016/j.jcou.2022.102050},
volume = {61},
year = {2022}
}
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RIS format (EndNote, RefMan)

TY  - JOUR
AB  - Dry reforming of methane (DRM) promises to reduce greenhouse gas emission by converting CO2 and CH4 (produced e.g. in anaerobic digestion processes) into syngas with an almost equimolar H2/CO ratio suitable for use in Fischer-Tropsch (FT) synthesis for the production of varieties of high value chemicals and liquid fuels. Ni-based catalyst is the most viable catalyst to catalyse the reaction, but its use faces a great challenge due to its propensity to form and accumulate carbonaceous materials on its active surface. In this article, the mechanisms involved in the deactivation of Ni-based catalyst in DRM reaction by carbon deposition and other carbon-induced deactivation mechanisms, which understanding is vital for the improvement of the process, are reviewed. Based on a thorough assessment of literature, perspectives are given on ways to control and mitigate carbon deposition problems related to the use of Ni-based catalysts in DRM by means of manipulating reaction conditions and process parameters as well as through designing and developing highly active coke-resistant Ni-based catalysts.
AU  - Baharudin,L
AU  - Rahmat,N
AU  - Othman,NH
AU  - Shah,N
AU  - Syed-Hassan,SSA
DO  - 10.1016/j.jcou.2022.102050
PY  - 2022///
SN  - 2212-9820
TI  - Formation, control, and elimination of carbon on Ni-based catalyst during CO<inf>2</inf>and CH<inf>4</inf>conversion via dry reforming process: A review
T2  - Journal of CO2 Utilization
UR  - http://dx.doi.org/10.1016/j.jcou.2022.102050
VL  - 61
ER  -
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