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• Journal article
  Guo K, Grunberg R, Ren Y, Chang T, Wustoni S, Strnad O, Koklu A, Diaz-Galicia E, Agudelo JP, Druet V, Castillo TCH, Moser M, Ohayon D, Hama A, Dada A, Mcculloch I, Viola I, Arold ST, Inal Set al., 2023,

  SpyDirect: A Novel Biofunctionalization Method for High Stability and Longevity of Electronic Biosensors

  , ADVANCED SCIENCE
  • Cite
• Journal article
  Liu T, Heimonen J, Zhang Q, Yang C-Y, Huang J-D, Wu H-Y, Stoeckel M-A, van der Pol TPA, Li Y, Jeong SY, Marks A, Wang X-Y, Puttisong Y, Shimolo AY, Liu X, Zhang S, Li Q, Massetti M, Chen WM, Woo HY, Pei J, McCulloch I, Gao F, Fahlman M, Kroon R, Fabiano Set al., 2023,

  Ground-state electron transfer in all-polymer donor:acceptor blends enables aqueous processing of water-insoluble conjugated polymers

  , NATURE COMMUNICATIONS, Vol: 14
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• Journal article
  Xu J, Spaeth A, Gruber W, Barabash A, Stadler P, Gubanov K, Wu M, Forberich K, Spiecker E, Fink RH, Unruh T, McCulloch I, Brabec CJ, Heumueller Tet al., 2023,

  Tailoring doped organic nanoparticles as selective hole transporters for printed non-fullerene organic solar cells

  , NANO ENERGY, Vol: 118, ISSN: 2211-2855
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• Journal article
  Zhong Y, Nayak PD, Wustoni S, Surgailis J, Agudelo JZP, Marks A, McCulloch I, Inal Set al., 2023,

  Ionic Liquid Gated Organic Electrochemical Transistors with Broadened Bandwidth

  , ACS APPLIED MATERIALS & INTERFACES, ISSN: 1944-8244
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• Journal article
  Savva A, Hama A, Herrera-Lopez G, Schmidt T, Migliaccio L, Steiner N, Kawan M, Fiumelli H, Magistretti PJ, Mcculloch I, Baran D, Gasparini N, Schindl R, Glowacki ED, Inal Set al., 2023,

  Photo-Chemical Stimulation of Neurons with Organic Semiconductors

  , ADVANCED SCIENCE, Vol: 10
  • Cite
  • Citations: 19
• Journal article
  Simatos D, Jacobs IE, Dobryden I, Nguyen M, Savva A, Venkateshvaran D, Nikolka M, Charmet J, Spalek LJ, Gicevicius M, Zhang Y, Schweicher G, Howe DJ, Ursel S, Armitage J, Dimov IB, Kraft U, Zhang W, Alsufyani M, Mcculloch I, Owens RM, Claesson PM, Knowles TPJ, Sirringhaus Het al., 2023,

  Effects of Processing-Induced Contamination on Organic Electronic Devices

  , SMALL METHODS, Vol: 7, ISSN: 2366-9608
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  • Citations: 8
• Journal article
  McCulloch I, Chabinyc M, Brabec C, Nielsen CB, Watkins SEet al., 2023,

  Sustainability considerations for organic electronic products

  , NATURE MATERIALS, Vol: 22, Pages: 1304-1310, ISSN: 1476-1122
  • Cite
  • Citations: 60
• Journal article
  Chen Y, Wang H, Chen H, Zhang W, Xu S, Paetzel M, Ma C, Wang C, McCulloch I, Hecht S, Samori Pet al., 2023,

  Quasi-1D Polymer Semiconductor - Diarylethene Blends: High Performance Optically Switchable Transistors

  , ADVANCED FUNCTIONAL MATERIALS, Vol: 33, ISSN: 1616-301X
  • Cite
  • Citations: 4
• Journal article
  Le VN, Bombile JH, Rupasinghe GS, Baustert KN, Li R, Maria IP, Shahi M, Alarcon Espejo P, McCulloch I, Graham KR, Risko C, Paterson AFet al., 2023,

  New Chemical Dopant and Counterion Mechanism for Organic Electrochemical Transistors and Organic Mixed Ionic-Electronic Conductors

  , ADVANCED SCIENCE, Vol: 10
  • Cite
  • Citations: 12
• Journal article
  Craighero M, Guo J, Zokaei S, Griggs S, Tian J, Asatryan J, Kimpel J, Kroon R, Xu K, Reparaz JS, Martin J, Mcculloch I, Campoy-Quiles M, Mueller Cet al., 2023,

  Impact of Oligoether Side-Chain Length on the Thermoelectric Properties of a Polar Polythiophene

  , ACS APPLIED ELECTRONIC MATERIALS, Vol: 6, Pages: 2909-2916
  • Cite
  • Citations: 15
• Journal article
  Ling Z, Nugraha MI, Hadmojo WT, Lin Y, Jeong SY, Yengel E, Faber H, Tang H, Laquai F, Emwas A-H, Chang X, Maksudov T, Gedda M, Woo HY, Mcculloch I, Heeney M, Tsetseris L, Anthopoulos TDet al., 2023,

  Over 19% Efficiency in Ternary Organic Solar Cells Enabled by n-Type Dopants

  , ACS ENERGY LETTERS, Vol: 8, Pages: 4104-4112, ISSN: 2380-8195
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• Journal article
  Druet V, Ohayon D, Petoukhoff CE, Zhong Y, Alshehri N, Koklu A, Nayak PD, Salvigni L, Almulla L, Surgailis J, Griggs S, McCulloch I, Laquai F, Inal Set al., 2023,

  A single n-type semiconducting polymer-based photo-electrochemical transistor

  , NATURE COMMUNICATIONS, Vol: 14
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• Journal article
  Keene ST, Laulainen JEM, Pandya R, Moser M, Schnedermann C, Midgley PA, McCulloch I, Rao A, Malliaras GGet al., 2023,

  Hole-limited electrochemical doping in conjugated polymers

  , NATURE MATERIALS, Vol: 22, Pages: 1121-+, ISSN: 1476-1122
  • Cite
  • Citations: 68
• Journal article
  Siemons N, 2023,

  Controlling swelling in mixed transport polymers through alkyl side-chain physical cross-linking

  , Proceedings of the National Academy of Sciences of USA, Vol: 120, ISSN: 0027-8424

  Semiconducting conjugated polymers bearing glycol side chains can simultaneously transport both electronic and ionic charges with high charge mobilities, making them ideal electrode materials for a range of bioelectronic devices. However, heavily glycolated conjugated polymer films have been observed to swell irreversibly when subjected to an electrochemical bias in an aqueous electrolyte. The excessive swelling can lead to the degradation of their microstructure, and subsequently reduced device performance. An effective strategy to control polymer film swelling is to copolymerize glycolated repeat units with a fraction of monomers bearing alkyl side chains, although the microscopic mechanism that constrains swelling is unknown. Here we investigate, experimentally and computationally, a series of archetypal mixed transporting copolymers with varying ratios of glycolated and alkylated repeat units. Experimentally we observe that exchanging 10% of the glycol side chains for alkyl leads to significantly reduced film swelling and an increase in electrochemical stability. Through molecular dynamics simulation of the amorphous phase of the materials, we observe the formation of polymer networks mediated by alkyl side-chain interactions. When in the presence of water, the network becomes increasingly connected, counteracting the volumetric expansion of the polymer film.

  • Abstract
  • Publisher Web Link
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• Conference paper
  Almulla L, Inal S, Petoukhoff CE, Alshehri N, Koklu A, Griggs S, Druet V, Alsufyani M, Yue W, McCulloch I, Laquai F, Wang Yet al., 2023,

  Soft Photosensitive Polymers as Water-Compatible Photodetectors

  , MATSUS Fall 2023 Conference, Publisher: FUNDACIO DE LA COMUNITAT VALENCIANA SCITO
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